Final Thoughts on Chemistry for 14564-35-3

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Organometallic Lewis Acids, IL. – Bis(acyl)-Bridged Heterometallic Complexes of Rhenium, Molybdenum, Ruthenium, and Copper

The reaction of the metalla-beta-diketonate complex <(OC)4-Re<-C(Me)O>2> with various organometallic Lewis acids yields the bis(acyl)-bridged bimetallic complexes (OC)4-Re<-C(Me)O->2Re(CO)4 (1), (OC)4Re<-C(Me)O->2MoCp(CO)2 (2), (OC)4Re<-C(Me)O->2Ru(eta3-C3H5)(nbd) (nbd = norbornadiene) (3), <(OC)4Re<-C(Me)O->2Ru(PPh3)2(CO)2> (4) and (OC)4Re<-C(Me)O->2Re(CO)4 (5), respectively.The structures of the compound 1-5 have been determined by X-ray diffraction.They show different conformations of the six-membered ring Re<-C(Me)O->2.The molecular structure of complex 1 proves a “flipping” of the acyl ligands. Key Words: Bis(acyl)-bridged bimetallic complexes / Rhenium complexes / Molybdenum complex / Ruthenium complex / Copper complex

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Highly efficient and robust molecular ruthenium catalysts for water oxidation,
Catalysts | Special Issue : Ruthenium Catalysts – MDPI