A new application about 138984-26-6

Here is just a brief introduction to this compound(138984-26-6)SDS of cas: 138984-26-6, more information about the compound(Dirhodium(II) tetrakis(caprolactam)) is in the article, you can click the link below.

In general, if the atoms that make up the ring contain heteroatoms, such rings become heterocycles, and organic compounds containing heterocycles are called heterocyclic compounds. An article called Divergent Rhodium-Catalyzed Cyclization Reactions of Enoldiazoacetamides with Nitrosoarenes, published in 2017-07-26, which mentions a compound: 138984-26-6, Name is Dirhodium(II) tetrakis(caprolactam), Molecular C24H40N4O4Rh2, SDS of cas: 138984-26-6.

The first cyclization reactions of enoldiazo compounds with nitrosoarenes have been developed. Under the catalysis of rhodium(II) octanoate, [3+2]-cyclization between enoldiazoacetamides and nitrosoarenes occurred through cleavages of the enol double bond and the amide bond, thus furnishing fully substituted 5-isoxazolone derivatives I [NR2 = piperidino, NMe2, R1 = Ph, 4-ClC6H4, 3-MeOC6H4, 2-MeC6H4, etc., R2 = SiMe2CMe3, Si(CHMe2)2]. Upon changing the catalyst to rhodium(II) caprolactamate, the reaction pathway switched to an unprecedented formal [5+1]-cyclization that provided multifunctionalized 1,3-oxazin-4-ones II with near exclusivity under otherwise identical conditions. Mechanistic studies uncovered distinct catalytic activities and reaction intermediates, which plausibly rationalized the novel reactivity and catalyst-controlled chemodivergence. Furthermore, a mechanism-inspired enantioselective rhodium-catalyzed reaction of γ-substituted enoldiazoacetamide with nitrosobenzene produced highly enantioenriched heterocycle-linked trialkylamine.

Here is just a brief introduction to this compound(138984-26-6)SDS of cas: 138984-26-6, more information about the compound(Dirhodium(II) tetrakis(caprolactam)) is in the article, you can click the link below.

Reference:
Highly efficient and robust molecular ruthenium catalysts for water oxidation,
Catalysts | Special Issue : Ruthenium Catalysts – MDPI